Magnetic susceptibility of ferrofluids determined from diffusion coefficient of a tracer
DOI:
https://doi.org/10.31349/RevMexFis.68.031003Keywords:
magnetic susceptibility, ferrofluid, magnetic, nanoparticles, linear response method, diffusion coefficient, dielectric relaxationAbstract
Linear response methods allow studying magnetic susceptibility relaxation in isotropic colloidal magnetic fluids. We show a relationship between the susceptibility of macroscopic magnetization at thermal equilibrium and the diffusion constant of a tracer particle. The comparison of the predicted frequency-dependent susceptibility with computer simulations shows their agreement. Besides, at a low concentration of particles, it has the expected Debye behavior. However, the initial susceptibility yields only the qualitative trends of the existing experiments at a low volume fraction of particles and its temperature dependence.
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